Author: ["G. P. Zhang","W. Hübner","Georgios Lefkidis","Yihua Bai","Thomas F. George"]
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Abstract
Conventional understanding of the magneto-optical Kerr effect, in which changes in the magnetization of a material cause changes in the polarization of reflected light, assumes that this incident light is continuous. However, first-principles simulations of nickel show that this assumption breaks down for femtosecond pulses of light, and establishes a firm foundation for understanding the dynamics of femtomagnetism. The magneto-optical Kerr effect (MOKE) is a powerful tool for studying changes in the magnetization of ferromagnetic materials. It works by measuring changes in the polarization of reflected light. However, because the conventional theoretical basis for interpreting a MOKE signal assumes measurement with continuous-wave light1,2, its use for understanding high-speed magnetization dynamics of a material probed with femtosecond optical pulses3,4 has been controversial5,6,7,8,9,10. Here we establish a new paradigm for interpreting time-resolved MOKE measurements, through a first-principles investigation of ferromagnetic nickel. We show that the time-resolved optical and magnetic responses energetically follow their respective optical and magneto-optical susceptibilities. As a result, the one-to-one correspondence between them sensitively depends on the incident photon energy. In nickel, for photon energies below 2 eV the magnetic response is faithfully reflected in the optical response, but above 2 eV they decouple. By constructing a phase-sensitive polarization versus magnetization plot, we find that for short pulses the magnetic signals are delayed by 10 fs with respect to the optical signals. For longer pulses, the delay shortens and the behaviour approaches the continuous-wave response. This finally resolves the long-standing dispute over the interpretation in the time-resolved MOKE measurements and lays a solid foundation for understanding femtomagnetism3,4.Cite this article
Zhang, G., Hübner, W., Lefkidis, G. et al. Paradigm of the time-resolved magneto-optical Kerr effect for femtosecond magnetism. Nature Phys 5, 499–502 (2009). https://doi.org/10.1038/nphys1315 