Evolution of the electronic excitation spectrum with strongly diminishing hole density in supercondu

Abstract

Coulomb interactions between the carriers may provide the mechanism for enhanced unconventional superconductivity in the copper oxides. However, they simultaneously cause inelastic quasiparticle scattering that can destroy it. Understanding the evolution of this balance with doping is crucial because it is responsible for the rapidly diminishing critical temperature as the hole density p is reduced towards the Mott insulating state. Here, we use tunnelling spectroscopy to measure the T→0 spectrum of electronic excitations N(E) over a wide range of hole density p in superconducting Bi2Sr2CaCu2O8+δ. We introduce a parameterization for N(E) based on a particle–hole symmetric anisotropic energy gap Δ(k)=Δ1(cos(kx)−cos(ky))/2 plus an inelastic scattering rate that varies linearly with energy Γ2(E)=α E. We demonstrate that this form of N(E) enables successful fitting of differential tunnelling conductance spectra throughout much of the Bi2Sr2CaCu2O8+δ phase diagram. We find that Δ1 values rise with falling p along the familiar trajectory of excitations to the ‘pseudogap’ energy, whereas the energy-dependent inelastic scattering rate Γ2(E)=α E seems to be an intrinsic property of the electronic structure and rises steeply for p<16%. Such diverging inelastic scattering may play a key role in suppression of superconductivity in the copper oxides as the Mott insulating state is approached. In conventional superconductors, the critical temperature goes to zero as the density of charge carriers falls due to increased scattering. But in high-temperature superconductors, the scattering rate as a function of charge carriers was unknown, until now.

Cite this article

Alldredge, J., Lee, J., McElroy, K. et al. Evolution of the electronic excitation spectrum with strongly diminishing hole density in superconducting Bi₂Sr₂CaCu₂O_8+δ. Nature Phys 4, 319–326 (2008). https://doi.org/10.1038/nphys917

View full text

>> Full Text:   Evolution of the electronic excitation spectrum with strongly diminishing hole density in supercondu