Confluence of resonant laser excitation and bidirectional quantum-dot nuclear-spin polarization

Abstract

Resonant laser scattering along with photon correlation measurements established the atom-like character of quantum dots. Here, we show that for a wide range of experimental parameters it is impossible to isolate elementary quantum-dot excitations from a strong influence of nuclear spins; the absorption lineshapes at magnetic fields exceeding 1 T indicate that the nuclear spins get polarized by an amount that ensures locking of the quantum-dot resonance to the incident laser frequency. In stark contrast to earlier experiments, this nuclear-spin polarization is bidirectional, allowing the combined electron–nuclear-spin system to track the changes in laser frequency dynamically on both sides of the resonance. This unexpected feature stems from a competition between two spin-pumping processes that attempt to polarize nuclear spins in opposite directions. We find that the confluence of laser excitation and nuclear-spin polarization suppresses the fluctuations in resonant absorption. A master-equation analysis suggests narrowing of the nuclear-spin distribution, pointing to applications in quantum information processing. In semiconductor quantum dots, interactions between the confined electrons and the surrounding reservoir of nuclear spins limit the attainable electron-spin coherence. But the nuclear-spin reservoir can also take a constructive role, as it facilitates the locking of the optical quantum-dot resonance to the changing frequency of an external driving laser, as an experiment now demonstrates.

Cite this article

Latta, C., Högele, A., Zhao, Y. et al. Confluence of resonant laser excitation and bidirectional quantum-dot nuclear-spin polarization. Nature Phys 5, 758–763 (2009). https://doi.org/10.1038/nphys1363

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